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ISSN: 2666-5549

Skeletal editing of pyridine for ring transformations

The pyridine ring, functioning as a vital framework in numerous bioactive molecules, has recently witnessed significant advancements in precise skeletal editing, which has brought about a revolutionary...

Advanced green synthesis: Solvent-free and catalyst-free reaction

The solvent-free and catalyst-free (SFCF) reaction has garnered significant interest among chemists due to its alignment with many of the 12 principles of green chemistry. In recent years, numerous...

Transaminase catalyzed asymmetric synthesis of active pharmaceutical ingredients

Chiral amine molecules constitute vital components of pharmaceutical ingredients. Recent years have witnessed a growing focus on the efficient synthesis of chiral amines. Transaminases, as catalysts,...

Intelligent enzyme design and hybrid catalytic systems: Driving innovation in biocatalysis

Enzyme engineering has emerged as a pivotal technology driving advances in biocatalysis, environmental remediation, and green chemistry. It is undergoing a transformative shift, propelled by the synergistic...

Perspectives on green synthesis and catalysis

Despite their impressive capacity to access diverse functional groups and to synthesize structurally complex molecules, the majority of the organic reactions suffers from harsh conditions, low atom...

Recent advances in the syntheses of pyrroles

The pyrrole moiety is an important structural motif in functional materials, natural products, and pharmaceuticals. More and more synthetic strategies toward pyrroles have emerged, where various efficient...

Visible-light induced site-selective C(sp3) –H epoxidation of amides

Oxiranes are among the most valuable reagents in the chemical sciences, with applications that span pharmaceuticals, agrochemicals, and functional materials. Although remarkable progress has been achieved...

Selective mono-methylation of primary alcohols and amines with methanol catalyzed by two-dimensional NHC–Ir coordination assemblies

Methanol, as a low-cost, abundant, and sustainable C1 feedstock, has garnered considerable attention for methylation reactions via the borrowing hydrogen (BH) process. Herein, we designed and synthesized...

Recent advances in ligand-accelerated nickel-catalyzed carbonylation under CO gas

Carbonyl groups are fundamental structural motifs in organic chemistry, prominently featured in drug molecules, functional materials, and as versatile synthetic intermediates. Transition metal-catalyzed...

Green polyurethanes from bio-based building blocks: Recent advances and applications

Polyurethanes (PUs) are among the most studied, manufactured, and employed polymers due to their versatility and wide range of applications. However, their synthesis generally relies on toxic, non-renewable,...

Photo-free electron donor-acceptor complexes driven divergent synthesis of thioethers and thioimidate esters with aryldiazonium salts and thiols/thiophenols

A catalyst- and photo-free strategy for the divergent synthesis of thioethers and thioimidate esters from thiophenols/thiols and aryldiazonium salts has been developed. The reaction pathway is precisely...

Recent advances in C–B bond formation by borylation with NHC–boranes

Organoboron compounds play a pivotal role in synthetic, pharmaceutical, and material chemistry due to their distinctive properties. Developing efficient, regioselective methods for C–B bond construction...

Chemo- and site-selective aerobic oxidation of methylbenzenes to aromatic aldehydes enabled by an Fe(III) photocatalyst

We have developed a chemo- and site-selective aerobic oxidation of methylbenzenes to aromatic aldehydes. It offers several advantages, including the use of an environmentally friendly catalyst (5 ​mol%...

CO2 hydrogenation to methanol on the incapsulated Cu-Zn catalyst: Effect of the MCM-41 and SBA-15 supports and the method of preparation on catalytic activity

The catalytic conversion of carbon dioxide to methanol is of great practical and scientific importance in the concept of reducing CO2 emissions. Moreover, it can partially solve the problem of human...

Recent advances in biocatalytic production of sugar acids

Sugar acids, as carbohydrate derivatives, are widely used in pharmaceuticals, food, and materials. Traditional chemical catalytic production methods can no longer meet the requirements for economic...

Metal-free electrochemical synthesis of sulfinamides via alkyl radical addition to sulfinylamines

Sulfinamides are important sulfur-containing motifs with broad applications in pharmaceuticals, agrochemicals, and materials. Traditional alkyl sulfinamide synthesis often requires prefunctionalized...

Lewis acid-catalyzed [4π+2σ] cycloaddition of bicyclo[2.1.0]pentanes with nitrones: Access to 2-oxa-3-azabicyclo[3.2.1]octanes

The hetero-bicyclo[3.2.1]octane scaffold is a prevalent structural motif in bioactive natural products and pharmaceuticals, yet general synthetic methods for its construction remain limited. Herein,...

Biotechnological synthesis of nucleoside analogs: Recent progress and perspectives

Nucleoside analogs play an indispensable role in antiviral and anticancer therapies, and improving their synthesis methods has become a focal area of research. In recent years, technological breakthroughs...

Recent advances in the electrochemical synthesis of oligosaccharides and glycosides

Sugars are fundamental building blocks in biological molecules such as oligosaccharides, glycoproteins, and glycosylated natural products. The construction of glycosidic bonds in a diastereoselective...

“Control from root design”: A proactive strategy for green and sustainable API process research and development

We detail the concept, implementation, and illustrative applications of the “control from root design” (CRD) strategy for developing safe, environmentally benign, simple, health-protective, quality-assured,...

Recent advances in the photocatalytic applications of ethyl bromodifluoroacetate: A review

Organic compounds bearing fluorine atoms have received widespread attention in recent years owing to their specific bioactivity and good biocompatibility compared to their nonfluorinated counterparts....

Contamination and biotransformation of deoxynivalenol (DON) in common commercial foods: Current status, challenges, and future perspectives

Deoxynivalenol (DON) has received considerable attention due to its toxicity and widespread presence in food and feed. This review summarizes the DON contamination in commonly consumed commercially...

Recent advances in transition-metal-free conversion of aldehydes to ketones

The preparation of functionalized ketones occupies an important position in synthetic organic chemistry because ketones are ubiquitous structural motifs in a broad range of compounds with various applications....

Unsaturated C2 synthons in photocatalysis: Taming and directing acetylene and ethylene in radical reactions

The conversion of the simplest unsaturated C2 molecular building units (C2H2 and C2H4) to high-value-added fine chemicals has been a pivotal domain in modern synthetic chemistry. Because of the inherent...

TBADT/nickel co-catalyzed three-component radical acylarylation of alkenes with aldehydes and aryl iodides

Here we report a photo/nickel co-catalyzed three-component acylarylation of alkenes using aldehydes and aryl iodides. Tetrabutylammonium decatungstate (TBADT) serves as a hydrogen-atom-transfer (HAT)...

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